The excited state electronic distribution and transport pathways in the COFs are probed using a host of experimental methods and theoretical calculations at a molecular level. Herein, we use reticular chemistry to construct a family of isoreticular crystalline hydrazide-based COF photocatalysts, with the optoelectronic properties and local pore characteristics of the COFs modulated using different linkers. However, their complicated structures lead to indeterminacy about photocatalytic active sites and reaction mechanisms. Covalent organic frameworks (COFs) represent an emerging class of organic photocatalysts.
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